Search results for "electronic topological"

showing 3 items of 3 documents

Structural and electrical study of the topological insulator SnBi2Te4 at high pressures

2016

We report high-pressure X-ray diffraction and electrical measurements of the topological insulator SnBi2Te4 at room temperature. The pressure dependence of the structural properties of the most stable phase of SnBi2Te4 at ambient conditions (trigonal phase) have been experimentally determined and compared with results of our ab initio calculations. Furthermore, a comparison of SnBi2Te4 with the parent compound Bi2Te3 shows that the central TeSnTe trilayer, which substitutes the Te layer at the center of the TeBiTeBiTe layers of Bi2Te3, plays a minor role in the compression of SnBi2Te4. Similar to Bi2Te3, our resistance measurements and electronic band structure simulations in SnBi2Te4 at hi…

DiffractionElectronic topological transitionMaterials science02 engineering and technology01 natural sciencesAb initio quantum chemistry methodsPhase (matter)0103 physical sciencesMaterials ChemistryElectrical measurementsTopological insulators010306 general physicsElectronic band structureCondensed matter physicsMechanical EngineeringMetals and Alloys021001 nanoscience & nanotechnologyX-ray diffractionHigh pressureMechanics of MaterialsHigh pressureTopological insulatorFISICA APLICADAX-ray crystallographyTransport properties0210 nano-technology
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High-pressure/high-temperature phase diagram of zinc

2018

The phase diagram of zinc (Zn) has been explored up to 140 GPa and 6000K, by combining optical observations, x-ray diffraction, and ab initio calculations. In the pressure range covered by this study, Zn is found to retain a hexagonal close-packed (hcp) crystal symmetry up to the melting temperature. The known decrease of the axial ratio (c/a) of the hcp phase of Zn under compression is observed in x-ray diffraction experiments from 300K up to the melting temperature. The pressure at which c/a reaches root 3 (approximate to 10GPa) is slightly affected by temperature. When this axial ratio is reached, we observed that single crystals of Zn, formed at high temperature, break into multiple pol…

DiffractionPhase transitionMaterials sciencemeltingPOWDER DIFFRACTIONELECTRONIC TOPOLOGICAL TRANSITIONSThermodynamicschemistry.chemical_elementFOS: Physical sciences02 engineering and technologyCrystal structureZincDIAMOND-ANVIL CELL01 natural scienceshigh temperatureCondensed Matter::Materials ScienceX-RAY-DIFFRACTIONPhase (matter)Condensed Matter::Superconductivity0103 physical sciencesGeneral Materials Science010306 general physicsMELTING CURVEPhase diagramCondensed Matter - Materials ScienceAxial ratioSYNCHROTRONab initio calculationszincMaterials Science (cond-mat.mtrl-sci)021001 nanoscience & nanotechnologyCondensed Matter PhysicsCompression (physics)EQUATION-OF-STATEhigh pressurechemistryx-ray diffractionphase transitionZNMETALS0210 nano-technologyRESISTANCE
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Characterization and Decomposition of the Natural van der Waals SnSb2Te4 under Compression

2020

[EN] High pressure X-ray diffraction, Raman scattering, and electrical measurements, together with theoretical calculations, which include the analysis of the topological electron density and electronic localization function, evidence the presence of an isostructural phase transition around 2 GPa, a Fermi resonance around 3.5 GPa, and a pressure-induced decomposition of SnSb2Te4 into the high-pressure phases of its parent binary compounds (alpha-Sb2Te3 and SnTe) above 7 GPa. The internal polyhedral compressibility, the behavior of the Raman-active modes, the electrical behavior, and the nature of its different bonds under compression have been discussed and compared with their parent binary…

Phase transitionContext (language use)[CHIM.INOR]Chemical Sciences/Inorganic chemistry010402 general chemistry01 natural sciencesInorganic Chemistrysymbols.namesakeChemical structureCationsVan der Waalselectronic topologicalPhysical and Theoretical ChemistryCompressibility010405 organic chemistryChemistryCompressionDeformation0104 chemical scienceshigh pressuremetavalent bondingChemical physicsFISICA APLICADAMolecular vibration[PHYS.COND.CM-MS]Physics [physics]/Condensed Matter [cond-mat]/Materials Science [cond-mat.mtrl-sci]symbolsCondensed Matter::Strongly Correlated ElectronsFermi resonanceSnSb2Te4pressure-induced decompositionvan der Waals forceTernary operationRaman spectroscopyRaman scatteringbonding characterInorganic Chemistry
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